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Materials Science in Additive Manufacturing                          Natural composite filaments for 3D-Print




                         A                        B                       C











            Figure 8. Schematic outline of the filament extrusion process based on varying fiber content and varying fiber specification,  namely (A) pure PLA
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            filament, (B) PLA filament mix including thin and short fibers, and (C) PLA filament mix including thick and long fibers
                         A                      C                        D











                        B








            Figure 9. Orthotropic behavior in PLA specimens manufactured via the FDM process: (A) Mechanical test through the 3-point bending test rig,
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            (B)  print orientations for PLA specimens, (C) 3-point bending test results, and (D) numerical simulation results including fringe plots of von-Mises
            stress distribution – Copyright disclosure –.
            Abbreviations: FDM: Fused deposition modeling; PLA: Polylactic acid

            mechanical properties in this area involved PLA as polymer   be approximately 42% and 5% greater, respectively, than
            matrix material. One mode of failure, which is commonly   the properties observed in neat PLA components.  In
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            observed in NFRC, namely fiber pull-out, was also found   another study, the mechanical properties in terms of the
            to take place in NFRCF hence indicating poor adhesion   ultimate tensile strength and Young’s modulus of neat PLA
            prevailing between the fiber and matrix interface.  In some   filament were found to be around 57.5 MPa and 3200 MPa,
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            cases, it was also observed that the mechanical properties   respectively.  Similar properties involving filament with a
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            of biodegradable composites tend to be inferior to pure   combination of PLA, PHA, and 10 – 20% fiber content, on
            matrix material as a result of several factors pertaining to   the other hand, were found to be around 25 MPa and 3750
            the nature of natural fibers.  The characteristics of various   MPa, respectively. 72
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            types of NFRCFs manufactured from diverse types of   Similar to NFRC fabrication, the volume composition of
            natural fibers are presented in Table 4.           natural fibers by weight percentage had direct implications
              For instance, the tensile strength and tensile modulus   on the mechanical properties of NFRCFs. A  general
            in fiber-reinforced PLA composites comprising Kraft pine   decreasing trend in the mechanical properties of the fiber-
            lignin as fiber reinforcement were found to be around 48   reinforced composite filament was observed to occur with
            MPa and 2.36 GPa, respectively, while those comprising   increasing fiber content.  Identical observations were
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            flax fibers were found to be around 33 MPa and 3.4 GPa,   found during the mechanical characterization of palm fiber-
            respectively.  The mechanical properties in terms of their   reinforced polyhydroxyalkanoate (PF-PHA) composites
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            tensile modulus and tensile strength of natural fiber-  for 3D-printing filaments. In that study, the notable
            reinforced composite components produced from 3 mm   increase in the tensile strength was attributed to the strong
            PLA filament reinforced with flax fibers were found to   interaction observed between the fiber reinforcement and


            Volume 4 Issue 1 (2025)                         11                             doi: 10.36922/msam.8533
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