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Materials Science in

                                                                  Additive Manufacturing



                                        ORIGINAL RESEARCH ARTICLE
                                        Enhancing interlaminar adhesion in

                                        multi-material 3D printing: A study of
                                        conductive PLA and TPU interfaces through

                                        fused filament fabrication



                                        Guo Liang Goh , Samuel Lee , Shi Hui Cheng , Daniel Jee Seng Goh ,
                                                     1,2
                                                                  1
                                                                                1
                                                                                                   1
                                                                                                       1,2
                                                                                     3
                                        Pothunuri Laya , Van Pho Nguyen , Boon Siew Han , and Wai Yee Yeong *
                                                     2
                                                                     1,3
                                        1 School of Mechanical and Aerospace Engineering, Nanyang Technological University, Singapore
                                        2 Singapore Centre for 3D Printing, School of Mechanical and Aerospace Engineering, Nanyang
                                        Technological University, Singapore
                                        3 Schaeffler Hub for Advanced Research, Nanyang Technological University, Singapore
                                        Abstract
                                        In the rapidly expanding field of additive manufacturing, multi-material fused
                                        filament fabrication represents a frontier with vast potential for creating composite
                                        structures  that  blend  the  benefits  of  different  material  properties.  Interlaminar
                                        adhesion between dissimilar materials remains a challenge for the realization of
                                        multifunctional structure for practical use. This study investigates the interlaminar
            *Corresponding author:      adhesion between conductive polylactic acid and thermoplastic polyurethane,
            Wai Yee Yeong               materials representative of rigid and flexible characteristics, respectively. We present
            (wyyeong@ntu.edu.sg)        a comparative analysis of two adhesion enhancement approaches: the incorporation
            Citation: Goh GL, Lee S,    of mechanical interlocking features and the modification of surface roughness
            Cheng SH, et al. Enhancing   at the interface.  Through tensile testing, we evaluate the effectiveness of these
            interlaminar adhesion in multi-  methods against a benchmark coupon with unmodified interface. Micro-computed
            material 3D printing: A study
            of conductive PLA and TPU   tomography analysis, surface morphology analysis, and mechanical performance
            interfaces through fused filament   assessments elucidate the failure modes and provide insights into the interfacial
            fabrication. Mater Sci Add Manuf.   behavior of these interface designs. We found that the interface design with top
            2024;3(1):2672.
            doi: 10.36922/msam.2672     infill modification showed the highest interlaminar adhesion strength, with an
                                        improvement of at least 25% compared to the benchmark coupon. Our findings aim
            Received: January 8, 2024
                                        to inform the design and manufacturing practices in multi-material 3D printing and
            Accepted: February 2, 2024  to open new avenues for the development of multifunctional, composite 3D-printed
            Published Online: February 27, 2024  systems.
            Copyright: © 2024 Author(s).
            This is an Open-Access article   Keywords: 3D printing; Additive manufacturing; Multi-material; Polymer; Composite
            distributed under the terms of the
            Creative Commons Attribution   material; Adhesion; Interface
            License, permitting distribution,
            and reproduction in any medium,
            provided the original work is
            properly cited.             1. Introduction
            Publisher’s Note: AccScience
            Publishing remains neutral with   The advent of additive manufacturing, also known as 3D printing, has transformed
            regard to jurisdictional claims in
            published maps and institutional   the landscape of material science and engineering, propelling the innovation of
            affiliations.               new applications across a diverse range of industries such as printed electronics,



            Volume 3 Issue 1 (2024)                         1                       https://doi.org/10.36922/msam.2672
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